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http://www.movie-locations.com/movies/a/Avengers_2012
"The exterior of the secret S.H.I.E.L.D. facility is Atrisco Heritage Academy High School, 10800 Dennis Chavez Boulevard SW, southwest of Albuquerque, augmented with plenty of suitably hi-tech dressing, including a full-scale helicopter pad smack in the middle of the school’s quad.
Apart from New Mexico, the film was shot around Cleveland, Ohio, and the vast laboratory itself is the122-feet high aluminium vacuum chamber of NASA’s Space Power facility, Plum Brook Station, in Sandusky, about 65 miles west of Cleveland."
It was in Avengers!